Statement of Yuri Dublyansky
IEER Press Conference
December 1, 1998, National Press Club
My name is Yuri Dublyansky, and I am Senior Scientist at the Institute
of Geology, Geophysics and Mineralogy of the Siberian Branch of a
Russian Academy of Sciences. My field of expertise is fluid inclusions
in minerals. I have been studying Yucca Mountain since 1994. Initially I
did so as a consultant to the State of Nevada.
According to the current concept a repository is proposed to be
constructed within the unsaturated zone of Yucca Mountain that is, in
relatively dry rocks, far above the water table. Regulations require
that the repository ensures safe containment of radionuclides for at
least 10,000 years. Peak radiation doses are expected to occur on far
longer time scales. In order to be able to forecast repository
performance in the future, we need to carefully understand the geologic
history of Yucca Mountain.
The concept of a high-level nuclear waste repository at Yucca Mountain
critically relies on the assumption that the repository zone will remain
unsaturated during the time period required for protection of the public
(on the order of tens of thousands of years). Therefore, an indication
that the mountain may have been saturated in the geologic past would be
very troubling.
The first doubts regarding the long-term stability of the unsaturated
zone at Yucca Mountain were raised as early as 1987 by the DOE Yucca
Mountain Project staff geologist J. Szymanski. His hypothesis regarding
the possibility of excursions of thermal waters into the currently
unsaturated zone was criticized and eventually discarded by a National
Research Council Panel in 1992.
The DOE and its contractors remain publicly confident that Yucca
Mountain has been unsaturated for millions of years and therefore that
the future stability of the unsaturated zone is reasonably assured for
the relevant time periods. Specifically, according to the DOE, the
unsaturated zone at Yucca Mountain was formed 9-10 million years ago and
since that time the water table has never risen more than about 300 feet
above its present level (which is 1000 feet below the planned repository
horizon). Therefore, any flooding of the repository in the future is
deemed unlikely.
A potential stumbling-block for the DOE-endorsed concept was discovered
during extensive exploration drilling at Yucca Mountain. Cores recovered
from boreholes often contained veinlets of calcite - a mineral which is
practically always formed by precipitation from water. These veinlets
represented "footprints" of ancient waters that moved inside the
mountain in the past. In 1995-1997, when a 5 mile-long tunnel (called
Exploratory Study Facility or ESF) was excavated into Yucca Mountain,
many more occurrences of secondary minerals became available for study.
DOE researchers interpreted this calcite as being deposited in the
unsaturated zone by rain water percolating through interconnected
fractures and carrying dissolved calcium carbonate from overlying soils.
Calcite was extensively studied in terms of its stable (carbon, oxygen)
and radiogenic (strontium, uranium, thorium, lead) isotope compositions
to determine its origin. The problem with this methodology is that
isotopic methods, on their own, are not capable of distinguishing
between different origins of minerals. The only method which can provide
unequivocal determination of the origin - the fluid inclusion method -
has never been adequately applied in the DOE studies
Fluid inclusions are tiny vacuoles in minerals, filled with the liquids
from which minerals grow. If these fluids are trapped and sealed at
elevated temperatures, upon cooling to ambient temperature they form
tiny bubbles inside them. This stems from the physical properties of
liquids and solids: on cooling liquids trapped in the inclusion contract
faster than surrounding solid, the pressure in the vacuole decreases and
at a certain point homogeneous liquid (e.g., water) splits onto two
phases: liquid and vapor. This process is reversible: if we heat such
inclusions, the pressure inside will increase and at some temperature,
the bubble will disappear and fluid will become homogeneous. This
temperature reflects the temperature of the liquid from which the
crystal grew. Inclusions in minerals formed at low temperatures (less
than ~35-40oC) do not contain bubbles.
In June 1998, I collected samples covering all 5 miles of the ESF
tunnel, and in October I conducted a study on the fluid inclusions in
them. The report that we release today presents the results of this
study.
Examination of calcite samples from the ESF tunnel leads to two
principal conclusions:
- the studied calcite was formed by upwelling of water and not from
percolation of surface water; and
- the water that entered the Yucca Mountain repository area in the past
from below was at elevated temperatures.
The main evidence for these findings is as follows:
- Many fluid inclusions in samples from the ESF had vapor bubbles
formed in them. I obtained about 300 measurements of fluid inclusion
temperatures, which indicate temperature of ancient water of 35 to 75oC. Water with such temperature could not have come from surface
sources.
- In a few samples, traces of aromatic hydrocarbons were found in
all-gas inclusions. Aromatic hydrocarbons are heavy molecules that
could not have originated in surface sources. There is evidence of
hydrocarbons (natural gas) in the geologic media beneath Yucca Mountain
area. Hence, the trapped hydrocarbons provide supplementary, though at
present fragmentary, evidence of upwelling of water into the repository
horizon.
- Veins and crusts at Yucca Mountain contain other minerals in addition
to calcite, such as opal, quartz, and minor fluorite. These minerals
typically precipitate from warm or hot water. In particular, it is
extremely rare for quartz and fluorite to be formed from surface water
percolation. Hence, the presence of these minerals is strong evidence
of past presence of upwelling warm water in the Yucca Mountain area.
- Minerals formed in an unsaturated zone, that is, above the water
table, are typically deposited in laminated formations consisting of
millions of tiny crystals. For example, stalactites in caves are
created in this way. By contrast, large perfectly shaped crystals
require a saturated environment to form. The calcite at Yucca Mountain
often forms perfectly shaped individual crystals up to 1.5 cm in size,
clearly indicating that the mountain was, at some time in the past,
saturated.
My study also addresses the question of the age of the calcites, though
in less detail. The timing of the formation of the calcites is important
because it provides evidence of when the area was saturated and hence of
the probability of its becoming saturated in the future during the
period relevant to repository performance. The findings of my research
for the timing of past repository saturation are only tentative and
indicative. There are indications that the calcite may have been formed
in the recent geologic past (less than one million years ago). This is
a very complex and difficult area of work and considerable further
research is needed to clarify this crucial question.
The issue addressed by my research has direct and significant bearing on
the viability of the site as a potential host for the high-level nuclear
waste repository. The critical questions remaining to be resolved are:
- When did the upwelling happen?
- Did it happen as a one-stage process, or did water rise and recede
intermittently?
- If the upwelling occurred in pulses, what was the recurrence period of
these pulses and what was the duration of each pulse?
- How much water was involved?
- What was the spatial distribution of this upwelling?
- What was the cause of the upwelling?
Only when all these questions have been satisfactorily answered can we
address the ultimate question:
- Could the repository become submerged again in the future on time
scales comparable to those during which radiation doses could be
significant?
Without these answers, any assessment of the site viability will
necessarily be incomplete. It is clearly premature at present to declare
the site viable.
More data need to be acquired and analyzed in order to assess the
implications of the new findings for repository viability. This may be
accomplished through concerted efforts of researchers, involving:
a. Detailed fluid inclusion studies in calcite and other minerals from
Yucca Mountain. Such studies may provide important information on the
spatial structure of the ancient hydrological system;
b. Careful dating of calcite samples hosting fluid inclusions indicating
elevated entrapment temperatures, which would constrain timing of
ancient hydrothermal system; and
c. Detailed isotopic study of minerals, which could provide important
information on the origin of fluids and pattern of fluid migration.
Saturation of the Yucca Mountain repository after burial of highly
radioactive waste could cause the waste canisters to corrode far more
rapidly than if the mountain remained dry allowing the radioactive
materials to be carried away. Because of the great threat to the
environment and to human health that would be posed by such a situation,
further study is absolutely necessary.
|